Efficient table-top dual-wavelength beamline for ultrafast transient absorption spectroscopy in the soft X-ray region

Publication date
DOI http://dx.doi.org/10.1038/s41598-020-62461-6
Reference L. Barreau, A.D. Ross, S. Garg, P.M. Kraus, D.M. Neumark and S.R. Leone, Efficient table-top dual-wavelength beamline for ultrafast transient absorption spectroscopy in the soft X-ray region, Sci. Rep 10, (1), 5733: 1-9 (2020)
Group High-Harmonic Generation & EUV Science

We present a table-top beamline providing a soft X-ray supercontinuum extending up to 370 eV from high-order harmonic generation with sub-13 fs 1300 nm driving pulses and simultaneous production of sub-5 fs pulses centered at 800 nm. Optimization of high harmonic generation in a long and dense gas medium yields a photon flux of similar to 1.4 x 10(6) photons/s/1% bandwidth at 300 eV. The temporal resolution of X-ray transient absorption experiments with this beamline is measured to be 11 fs for 800 nm excitation. This dual-wavelength approach, combined with high flux and high spectral and temporal resolution soft X-ray absorption spectroscopy, is a new route to the study of ultrafast electronic dynamics in carbon-containing molecules and materials at the carbon K-edge.